• Media type: Text; E-Article
  • Title: Airborne concentrations and chemical considerations of radioactive ruthenium from an undeclared major nuclear release in 2017
  • Contributor: Masson, O. [Author]; Steinhauser, G. [Author]; Zok, D. [Author]; Saunier, O. [Author]; Angelov, H. [Author]; Babic, D. [Author]; Beckova, V. [Author]; Bieringer, J. [Author]; Bruggeman, M. [Author]; Burbidge, C.I. [Author]; Conil, S. [Author]; Dalheimer, A. [Author]; Geer, L.-E. [Author]; Ott, A. de Vismes [Author]; Eleftheriadis, K. [Author]; Estier, S. [Author]; Fischer, H. [Author]; Garavaglia, M.G. [Author]; Leonarte, C.G. [Author]; Gorzkiewicz, K. [Author]; Hainz, D. [Author]; Hoffman, I. [Author]; Hýža, M. [Author]; Isajenko, K. [Author]; [...]
  • Published: Washington, DC : NAS, 2019
  • Published in: Proceedings of the National Academy of Sciences of the United States of America (PNAS) 116 (2019), Nr. 34
  • Issue: published Version
  • Language: English
  • DOI: https://doi.org/10.15488/10953; https://doi.org/10.1073/pnas.1907571116
  • ISSN: 0027-8424
  • Keywords: environmental radioactivity ; ruthenium ; accidental release ; environmental release ; nuclear forensics
  • Origination:
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  • Description: A massive atmospheric release of radioactive 106Ru occurred in Eurasia in 2017, which must have been caused by a sizeable, yet undeclared nuclear accident. This work presents the most compelling monitoring dataset of this release, comprising 1,100 atmospheric and 200 deposition data points from the Eurasian region. The data suggest a release from a nuclear reprocessing facility located in the Southern Urals, possibly from the Mayak nuclear complex. A release from a crashed satellite as well as a release on Romanian territory (despite high activity concentrations) can be excluded. The model age of the radioruthenium supports the hypothesis that fuel was reprocessed ≤2 years after discharge, possibly for the production of a high-specific activity 144Ce source for a neutrino experiment in Italy.
  • Access State: Open Access
  • Rights information: Attribution - Non Commercial - No Derivs (CC BY-NC-ND)