• Media type: E-Article
  • Title: Chiral Unsymmetrically Substituted Bipyridine N,N′‐Dioxides as Catalysts for the Allylation of Aldehydes
  • Contributor: Ulč, Jan; Nečas, David; Koukal, Petr; Havlíček, Vojtěch; Tošner, Zdeněk; Hybelbauerová, Simona; Kotora, Martin
  • imprint: Wiley, 2018
  • Published in: European Journal of Organic Chemistry
  • Language: English
  • DOI: 10.1002/ejoc.201800485
  • ISSN: 1434-193X; 1099-0690
  • Origination:
  • Footnote:
  • Description: <jats:p>A series of unsymmetrically substituted diastereoisomeric (<jats:italic>R<jats:sub>a</jats:sub>,R</jats:italic>) and (<jats:italic>S<jats:sub>a</jats:sub>,R</jats:italic>) bipyridine <jats:italic>N</jats:italic>,<jats:italic>N′</jats:italic>‐dioxides was synthesized by using oxidative coupling of the corresponding metallated tetrahydroisoquinoline <jats:italic>N</jats:italic>‐oxides in the presence of iodine. The <jats:italic>N</jats:italic>,<jats:italic>N′</jats:italic>‐dioxides contained substituted aryl groups with electron‐donating or electron‐accepting groups in the near vicinity of the <jats:italic>N</jats:italic>,<jats:italic>N′</jats:italic>‐dioxide moiety. Their catalytic activity was tested in a series of reactions of allyltrichlorosilane with various substituted benzaldehydes, thiophenecarbaldehyde, and cinnamaldehyde. The reactions proceeded with high enantioselectivities (up to 98 % <jats:italic>ee</jats:italic>) with catalyst loadings as low as 0.5 mol‐%. Furthermore, allylation reactions of (<jats:italic>E</jats:italic>)‐3‐iodomethacrylaldehyde were also carried out to give chiral (<jats:italic>E</jats:italic>)‐1‐iodo‐2‐methylpenta‐1,4‐dien‐3‐ol, a convenient building block for the synthesis of natural products. The allylations proceeded with high enantioselectivities (up to ca. 99 % <jats:italic>ee</jats:italic>) with a catalyst loading of 2.5 mol‐%.</jats:p>