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Levin, Nikita; Margraf, Johannes T.; Lengyel, Jozef; Reuter, Karsten; Tschurl, Martin; Heiz, Ulrich

CO2-Activation by size-selected tantalum cluster cations (Ta1–16+): thermalization governing reaction selectivity

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  • Media type: E-Article
  • Title: CO2-Activation by size-selected tantalum cluster cations (Ta1–16+): thermalization governing reaction selectivity
  • Contributor: Levin, Nikita; Margraf, Johannes T.; Lengyel, Jozef; Reuter, Karsten; Tschurl, Martin; Heiz, Ulrich
  • Published: Royal Society of Chemistry (RSC), 2022
  • Published in: Physical Chemistry Chemical Physics, 24 (2022) 4, Seite 2623-2629
  • Language: English
  • DOI: 10.1039/d1cp04469a
  • ISSN: 1463-9084; 1463-9076
  • Keywords: Physical and Theoretical Chemistry ; General Physics and Astronomy
  • Origination:
  • Footnote:
  • Description: <jats:p>Tantalum cluster cations react with CO<jats:sub>2</jats:sub> either <jats:italic>via</jats:italic> transfer of oxygen atoms to the clusters or the adsorption of an entire molecule. The released energy and vibrational heat capacities are assigned to determine the branching ratios of the pathways.</jats:p>