• Media type: E-Article
  • Title: The Use of an Acylhydrazone-Based Metal-Organic Framework in Solid-Contact Potassium-Selective Electrode for Water Analysis
  • Contributor: Kościelniak, Paweł; Dębosz, Marek; Wieczorek, Marcin; Migdalski, Jan; Szufla, Monika; Matoga, Dariusz; Kochana, Jolanta
  • Published: MDPI AG, 2022
  • Published in: Materials, 15 (2022) 2, Seite 579
  • Language: English
  • DOI: 10.3390/ma15020579
  • ISSN: 1996-1944
  • Origination:
  • Footnote:
  • Description: A solid-contact ion-selective electrode was developed for detecting potassium in environmental water. Two versions of a stable cadmium acylhydrazone-based metal organic framework, i.e., JUK-13 and JUK-13_H2O, were used for the construction of the mediation layer. The potentiometric and electrochemical characterizations of the proposed electrodes were carried out. The implementation of the JUK-13_H2O interlayer is shown to improve the potentiometric response and stability of measured potential. The electrode exhibits a good Nernstian slope (56.30 mV/decade) in the concentration range from 10−5 to 10−1 mol L−1 with a detection limit of 2.1 µmol L−1. The long-term potential stability shows a small drift of 0.32 mV h−1 over 67 h. The electrode displays a good selectivity comparable to ion-selective electrodes with the same membrane. The K-JUK-13_H2O-ISE was successfully applied for the determination of potassium in three certified reference materials of environmental water with great precision (RSD < 3.00%) and accuracy (RE < 3.00%).
  • Access State: Open Access