> Detailanzeige

Fry, M.M. [VerfasserIn]; Naik, V. [VerfasserIn]; Duncan, B.N. [VerfasserIn]; Hess, P. [VerfasserIn]; MacKenzie, I.A. [VerfasserIn]; Marmer, E. [VerfasserIn]; Schultz, M.G. [VerfasserIn]; Szopa, S. [VerfasserIn]; Wild, O. [VerfasserIn]; Zeng, G. [VerfasserIn]; West, J.J. [VerfasserIn]; Schwarzkopf, M.D. [VerfasserIn]; Fiore, A.M. [VerfasserIn]; Collins, W.J. [VerfasserIn]; Dentener, F.J. [VerfasserIn]; Shindell, D.T. [VerfasserIn]; Atherton, C. [VerfasserIn]; Bergmann, D. [VerfasserIn]

The influence of ozone precursor emissions from four world regions on tropospheric composition and radiative climate forcing

Literatur-
verwaltung

Zur
Merkliste

Lösche von
Merkliste

Per Whatsapp teilen

Schließen

Merkliste



Sie können Bookmarks mittels Listen verwalten, loggen Sie sich dafür bitte in Ihr SLUB Benutzerkonto ein.
  • Medientyp: E-Artikel
  • Titel: The influence of ozone precursor emissions from four world regions on tropospheric composition and radiative climate forcing
  • Beteiligte: Fry, M.M. [VerfasserIn]; Naik, V. [VerfasserIn]; Duncan, B.N. [VerfasserIn]; Hess, P. [VerfasserIn]; MacKenzie, I.A. [VerfasserIn]; Marmer, E. [VerfasserIn]; Schultz, M.G. [VerfasserIn]; Szopa, S. [VerfasserIn]; Wild, O. [VerfasserIn]; Zeng, G. [VerfasserIn]; West, J.J. [VerfasserIn]; Schwarzkopf, M.D. [VerfasserIn]; Fiore, A.M. [VerfasserIn]; Collins, W.J. [VerfasserIn]; Dentener, F.J. [VerfasserIn]; Shindell, D.T. [VerfasserIn]; Atherton, C. [VerfasserIn]; Bergmann, D. [VerfasserIn]
  • Erschienen: Union, 2012
  • Erschienen in: Journal of Geophysical Research 117, 1 - 16 (2012). doi:10.1029/2011JD017134
  • Sprache: Englisch
  • DOI: https://doi.org/10.1029/2011JD017134
  • ISSN: 0141-8637; 0148-0227
  • Schlagwörter:
  • Entstehung:
  • Anmerkungen: Diese Datenquelle enthält auch Bestandsnachweise, die nicht zu einem Volltext führen.
  • Beschreibung: Ozone (O-3) precursor emissions influence regional and global climate and air quality through changes in tropospheric O-3 and oxidants, which also influence methane (CH4) and sulfate aerosols (SO42-). We examine changes in the tropospheric composition of O-3, CH4, SO42- and global net radiative forcing (RF) for 20% reductions in global CH4 burden and in anthropogenic O-3 precursor emissions (NOx, NMVOC, and CO) from four regions (East Asia, Europe and Northern Africa, North America, and South Asia) using the Task Force on Hemispheric Transport of Air Pollution Source-Receptor global chemical transport model (CTM) simulations, assessing uncertainty (mean +/- 1 standard deviation) across multiple CTMs. We evaluate steady state O-3 responses, including long-term feedbacks via CH4. With a radiative transfer model that includes greenhouse gases and the aerosol direct effect, we find that regional NOx reductions produce global, annually averaged positive net RFs (0.2 +/- 0.6 to 1.7 +/- 2 mWm(-2)/TgN yr(-1)), with some variation among models. Negative net RFs result from reductions in global CH4 (-162.6 +/- 2 mWm(-2) for a change from 1760 to 1408 ppbv CH4) and regional NMVOC (-0.4 +/- 0.2 to -0.7 +/- 0.2 mWm(-2)/Tg C yr(-1)) and CO emissions (-0.13 +/- 0.02 to -0.15 +/- 0.02 mWm(-2)/Tg CO yr(-1)). Including the effect of O-3 on CO2 uptake by vegetation likely makes these net RFs more negative by -1.9 to -5.2 mWm(-2)/Tg N yr(-1), -0.2 to -0.7 mWm(-2)/Tg C yr(-1), and -0.02 to -0.05 mWm(-2)/Tg CO yr(-1). Net RF impacts reflect the distribution of concentration changes, where RF is affected locally by changes in SO42-, regionally to hemispherically by O-3, and globally by CH4. Global annual average SO42- responses to oxidant changes range from 0.4 +/- 2.6 to -1.9 +/- 1.3 Gg for NOx reductions, 0.1 +/- 1.2 to -0.9 +/- 0.8 Gg for NMVOC reductions, and -0.09 +/- 0.5 to -0.9 +/- 0.8 Gg for CO reductions, suggesting additional research is needed. The 100-year global warming potentials (GWP(100)) are calculated for the global ...
  • Zugangsstatus: Freier Zugang