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Hockett, Paul; Reid, Katharine L.

Complete determination of the photoionization dynamics of a polyatomic molecule. II. Determination of radial dipole matrix elements and phases from experimental photoelectron angular distributions from ÃAu1 acetylene

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  • Medientyp: E-Artikel
  • Titel: Complete determination of the photoionization dynamics of a polyatomic molecule. II. Determination of radial dipole matrix elements and phases from experimental photoelectron angular distributions from ÃAu1 acetylene
  • Beteiligte: Hockett, Paul; Reid, Katharine L.
  • Erschienen: AIP Publishing, 2007
  • Erschienen in: The Journal of Chemical Physics, 127 (2007) 15
  • Sprache: Englisch
  • DOI: 10.1063/1.2790443
  • ISSN: 0021-9606; 1089-7690
  • Schlagwörter: Physical and Theoretical Chemistry ; General Physics and Astronomy
  • Entstehung:
  • Anmerkungen:
  • Beschreibung: <jats:p>We present a fit to photoelectron angular distributions (PADs) measured following the photoionization of rotationally selected ÃAu1 state acetylene. In the case of the 41Σu−2 vibronic state of the ion, we are able to use this fit to make a complete determination of the radial dipole matrix elements and phases connecting the prepared level to each photoelectron partial wave. We have also investigated other Renner-Teller subbands with a view to disentangling geometrical and dynamical contributions to the resulting PADs.</jats:p>